Title
Rotating wave approximation effects on the nonlinear optical responses of complex molecular systems using a four-wave mixing signal
Date Issued
12 March 2015
Access level
metadata only access
Resource Type
journal article
Author(s)
Universidad Simón Bolívar
Publisher(s)
Taylor and Francis Ltd.
Abstract
The study of a two-level molecular system with permanent dipole moments (PDM) immersed in a thermal bath and interacting with an electromagnetic field depends on the inclusion of the rotating wave approximation (RWA). A methodology based on cumulant expansions to obtain the average in the Fourier components associated with the coherences and populations, calculated by the optical stochastic Bloch equations, is employed. With these equations, we have modeled the optical responses for the four-wave mixing signal and we have demonstrated that inside the RWA the PDM cannot be measured.
Start page
403
End page
411
Volume
62
Issue
5
Language
English
OCDE Knowledge area
Óptica
Subjects
Scopus EID
2-s2.0-84937524523
Source
Journal of Modern Optics
ISSN of the container
09500340
Sponsor(s)
JLP, JFC-G, and LGR acknowledge the financial support provided by the SENESCYT-Ecuador through the Prometeo Project.
Sources of information:
Directorio de Producción Científica
Scopus