Title
Absorptive and dispersive optical profiles in fluctuating environments: A stochastic model
Date Issued
01 January 2011
Access level
metadata only access
Resource Type
journal article
Author(s)
Universidad Simón Bolívar
Abstract
In this study, we determined the absorptive and dispersive optical profiles of a molecular system coupled with a thermal bath. Solvent effects were explicitly considered by modelling the non-radiative interaction with the solute as a random variable. The optical stochastical Bloch equations (OSBE) were solved using a time-ordered cumulant expansion with white noise as a correlation function. We found a solution for the Fourier component of coherence at the third order of perturbation for the nonlinear Four-wave mixing signal and produced analytical expressions for the optical responses of the system. Finally, we examined the behaviour of these properties with respect to the noise parameter, frequency detuning of the dynamic perturbation, and relaxation times. © 2010 Elsevier Ltd.
Start page
100
End page
108
Volume
112
Issue
1
Language
English
OCDE Knowledge area
Óptica
Subjects
Scopus EID
2-s2.0-78049302038
Source
Journal of Quantitative Spectroscopy and Radiative Transfer
ISSN of the container
00224073
Sponsor(s)
This work was partially supported by Decanato de Investigación y Desarrollo of Universidad Simón Bolívar (Grant GID-13 ) and by Fondo Nacional de Ciencia, Tecnología e Innovación, FONACIT (Grant G-97000593 ).
Sources of information:
Directorio de Producción Científica
Scopus