Title
Theoretical framework for the interpretation of STM images of adsorbates
Date Issued
01 January 1992
Access level
metadata only access
Resource Type
journal article
Author(s)
University of Oregon
Abstract
A theoretical formalism for the interpretation of STM images of adsorbates is developed by approaching the calculation of the observed current as a transport problem in quantum statistical mechanics. The STM configuration is treated as a system of three groups of states - the substrate, the adsorbate and the tip - in contact with a thermal reservoir, with which it exchanges energy. A new definition of current is introduced, and shown to be related to that given in the traditional transfer Hamiltonian approach. The transport instrument used for the description is the stochastic Liouville equation, known to have the advantage of allowing the incorporation of thermal effects as well as arbitrary degree of coherence in the quantum transport. Some preliminary calculations of STM images of simple adsorbate models are presented. © 1992.
Start page
122
End page
127
Volume
42-44
Issue
PART 1
Language
English
OCDE Knowledge area
Física de la materia condensada
Nano-tecnología
Scopus EID
2-s2.0-0026898720
PubMed ID
Source
Ultramicroscopy
ISSN of the container
03043991
Sponsor(s)
This work was partially supportedb y NIH grant GM 32543, by NSF grant DIR-8820732 to C.B. and by an Institute of Molecular Biology Research Fellowship to F.B. We would also like to thank Dr. Dale Tronrud and Professor Brian Matthews for the use of their computing facilities and assistance.D r. Ricardo Garcia has stimulated useful discussions.
Sources of information:
Directorio de Producción Científica
Scopus