Title
Surface Phonon-Polariton Heat Capacity of Polar Nanofilms
Date Issued
01 May 2021
Access level
open access
Resource Type
journal article
Author(s)
The University of Tokyo
Publisher(s)
American Physical Society
Abstract
The surface phonon-polariton heat capacity of polar nanofilms is analytically determined and analyzed as a function of their thickness and temperature. It is shown that the polariton heat capacity increases with the square of the nanofilm thickness, such that for thin enough nanofilms at sufficient low temperature T, its value becomes independent of the material properties and is given by C=1.15ϵ0kB(kBT/ℏc)2, where ϵ0 and c are the respective relative permittivity of the surrounding medium and light speed in vaccum, while kB and 2πℏ are the Boltzmann and Planck constants, respectively. The photonlike nature of surface phonon polaritons is found to be responsible for their main contribution to the material heat capacity. As a result of the polariton speed close to c and hence much higher than that of phonons, the polariton heat capacity of SiO2, SiC, and SiN is found to be several orders of magnitude smaller than its corresponding phonon counterpart. Surface phonon polaritons are thus not expected to increase the expansion coefficient of polar nanofilms, which favors their utilization as effective heat dissipators.
Volume
15
Issue
5
Language
English
OCDE Knowledge area
Nano-materiales
Física de partículas, Campos de la Física
Scopus EID
2-s2.0-85107585538
Source
Physical Review Applied
Sources of information:
Directorio de Producción Científica
Scopus