Title
Solvent effects on the optical properties of two-level systems with permanent dipole moments
Date Issued
01 December 2013
Access level
metadata only access
Resource Type
conference paper
Author(s)
Universidad Simón Bolívar
Abstract
The inclusion of the permanent dipole moments and the solvent on the optical conventional Bloch equations (OCBE) allowed us to obtain analytical expressions for the optical properties of a two-level molecular system. We employed the methodology developed by Colmenares et al.1, in which they model the collisional effect of the solvent through a stochastical function, t ω0 σ t so the OCBE become a set of coupled integro-differential stochastical equations that we solved, up to third order in the incident field, employing the perturbation theory. Once obtained the analytical expressions for the density matrix elements, macroscopic polarization and effective susceptibility of the system, we studied the optical properties derived in the frequency space, inside and outside the rotating wave approximation. © 2013 SPIE.
Volume
8785
Language
English
OCDE Knowledge area
Óptica
Subjects
Scopus EID
2-s2.0-84891331534
Source
Proceedings of SPIE - The International Society for Optical Engineering
Resource of which it is part
Proceedings of SPIE - The International Society for Optical Engineering
ISSN of the container
1996756X
ISBN of the container
9780819496010
Sources of information:
Directorio de Producción Científica
Scopus