Title
Field-induced metamagnetic transitions and two-dimensional excitations in ludwigite Co 4. 76 Al 1. 24(O 2 BO 3) 2
Date Issued
26 June 2017
Access level
metadata only access
Resource Type
journal article
Author(s)
Freitas D.C.
Passamani E.C.
Pinheiro C.B.
Baggio-Saitovitch E.
Continentino M.A.
Sanchez D.R.
Universidade Federal Fluminense
Publisher(s)
American Physical Society
Abstract
This paper presents an extensive study of the structural, magnetic, and thermodynamic properties of the heterometallic ludwigite Co4.76Al1.24(O2BO3)2. This material orders ferrimagnetically at 57 K. Despite the fact that, in Co4.76Al1.24(O2BO3)2, one quarter of the Co ions of the parent compound Co3O2BO3 is replaced by nonmagnetic Al3+ ions, the TC of the former (57 K) is larger than that of the latter (42 K). We obtain the phase diagram of Co4.76Al1.24(O2BO3)2 in an external magnetic field. We find a line of second-order phase transitions where the system presents a metamagnetic transition (from 57 to 25 K). This line ends at a tricritical point at 25 K and 4.3 T, below which the transition to the paramagnetic phase is first order (from 25 to 3 K). In the magnetic phase at low temperatures specific heat measurements in zero and finite magnetic fields show that the low-energy excitations are magnetic (magnons) and elastic (phonons) excitations with two-dimensional character. These measurements also reveal the magnetocaloric properties of this material.
Volume
95
Issue
21
Language
English
OCDE Knowledge area
Física de partículas, Campos de la Física Física atómica, molecular y química
Scopus EID
2-s2.0-85023619559
Source
Physical Review B
ISSN of the container
24699950
Sponsor(s)
Support from the Brazilian agencies CNPq and FAPERJ is gratefully acknowledged. We also acknowledge LDRX-UFF (Universidade Federal Fluminense, Brazil) for use of their laboratory facilities.
Sources of information: Directorio de Producción Científica Scopus