Title
Onset of convection for autocatalytic reaction fronts: Laterally bounded systems
Date Issued
01 January 1991
Access level
open access
Resource Type
journal article
Author(s)
West Virginia University
Abstract
Linear hydrodynamics yields the onset of convection for ascending autocatalytic reaction fronts in laterally bounded geometries. The system is studied in the limit of infinite and zero thermal diffusivity. For convection in a vertical slab of thickness a or a long vertical cylinder of radius a, the appropriate dimensionless driving parameter scrS=ga3/Dc involves the fractional density difference between the unreacted and reacted fluids, the acceleration of gravity g, the kinematic viscosity , and the catalyst molecular diffusivity Dc. Calculated critical values scrSc for onset of convection agree with recent experiments on iodatearsenous acid systems. We also show that, compared with the unbounded system, the sidewalls tend to suppress convection. © 1991 The American Physical Society.
Start page
6694
End page
6699
Volume
43
Issue
12
Language
English
OCDE Knowledge area
Física de plasmas y fluídos
Scopus EID
2-s2.0-0039890647
Source
Physical Review A
ISSN of the container
10502947
Sources of information: Directorio de Producción Científica Scopus