Title
Electrical control of interlayer exciton dynamics in atomically thin heterostructures
Date Issued
15 November 2019
Access level
open access
Resource Type
journal article
Author(s)
Joe A.Y.
Pistunova K.
Wild D.S.
High A.A.
Zhou Y.
Scuri G.
de Greve K.
Sushko A.
Yu C.H.
Taniguchi T.
Watanabe K.
Needleman D.J.
Lukin M.D.
Park H.
Kim P.
University of California
Publisher(s)
American Association for the Advancement of Science
Abstract
A van der Waals heterostructure built from atomically thin semiconducting transition metal dichalcogenides (TMDs) enables the formation of excitons from electrons and holes in distinct layers, producing interlayer excitons with large binding energy and a long lifetime. By employing heterostructures of monolayer TMDs, we realize optical and electrical generation of long-lived neutral and charged interlayer excitons. We demonstrate that neutral interlayer excitons can propagate across the entire sample and that their propagation can be controlled by excitation power and gate electrodes. We also use devices with ohmic contacts to facilitate the drift motion of charged interlayer excitons. The electrical generation and control of excitons provide a route for achieving quantum manipulation of bosonic composite particles with complete electrical tunability.
Start page
870
End page
875
Volume
366
Issue
6467
Language
English
OCDE Knowledge area
IngenierÃa quÃmica
QuÃmica fÃsica
Scopus EID
2-s2.0-85075060829
PubMed ID
Source
Science
ISSN of the container
00368075
Sponsor(s)
This work is supported by the DoD Vannevar Bush Faculty Fellowship (N00014-18-1-2877 for P.K., N00014-16-1-2825 for H.P.), AFOSR MURI (FA9550-17-1-0002), NSF and CUA (PHY-1506284 and PHY-1125846 for H.P. and M.D.L.), ARL (W911NF1520067 for H.P. and M.D.L.), the Gordon and Betty Moore Foundation (GBMF4543 for P.K.), and Samsung Electronics (for P.K. and H.P.). This work was performed in part at the Center for Nanoscale Systems (CNS), a member of the National Nanotechnology Coordinated Infrastructure (NNCI), which is supported by the National Science Foundation under NSF award 1541959. CNS is part of Harvard University. D.J.N. acknowledges support from the NSF grant DBI-0959721. A.S. acknowledges support from the Fannie and John Hertz Foundation and the Paul & Daisy Soros Fellowships for New Americans. K.W. and T.T. acknowledge support from the Elemental Strategy Initiative conducted by the MEXT, Japan, and the CREST (JPMJCR15F3), JST. Author contributions: L.A.J., A.Y.J., and P.K. conceived the
Sources of information:
Directorio de Producción CientÃfica
Scopus