Title
Study of the absorptive and dispersive responses of molecular systems under stochastic considerations
Date Issued
25 September 2014
Access level
metadata only access
Resource Type
journal article
Author(s)
Mastrodomenico A.
Cárdenas-García J.F.
Rodriguez L.G.
Costa-Vera C.
Universidad Simón Bolívar
Publisher(s)
World Scientific Publishing Co. Pte Ltd
Abstract
Absorptive and dispersive nonlinear optical properties have been studied considering a two-level molecular system with permanent dipole moments immersed in a thermal reservoir interacting with a classical electromagnetic field. Our model is based in a stochastic description, where the system-solvent interaction induces random shifts in the Bohr frequency (ω0) that transforms ω0 into a stochastic variable ξ(t). Our results show that it is necessary to neglect the rotating-wave approximation in order to measure the effect of the permanent dipole moments. The two-photon transitions over those with one-photon are favored when the permanent dipole moments are considered.
Volume
23
Issue
3
Language
English
OCDE Knowledge area
Óptica
Scopus EID
2-s2.0-84928412988
Source
Journal of Nonlinear Optical Physics and Materials
ISSN of the container
02188635
Sponsor(s)
JLP, JFC-G and LGR acknowledge the financial support provided by the Secretaría Nacional de Educación Superior, Ciencia, Tecnología e Innovación (SENESCYT) of Ecuador through the Prometeo Fellowship. JLP also acknowledges the financial support of the Decanato de Investigación y Desarrollo of Universidad Simón Bolívar (Grant GID-013), Caracas, Venezuela.
Sources of information: Directorio de Producción Científica Scopus