Title
Absortive and dispersive optical properties in molecular systems
Date Issued
01 May 2009
Access level
metadata only access
Resource Type
journal article
Author(s)
Romero-Depablos A.
Gorayeb M.
Castro E.
Martín P.
Universidad Simón Bolívar
Abstract
Solute-solvent collisions for a two-level molecular system interacting with a four-wave mixing signal are analyzed in the present contribution. The system is described using the optical stochastic Bloch equations (OSBE), where Bohr's frequency is treated a stochastic variable due to the random collisions with the solvent. The resulting equations for the Fourier components associated to the coherence are averaged over all the realizations of the stochastic variable, using an approximant for the Voigt's function as a probability distribution. In this model we were able to calculate the optical susceptibilities at different frequencies, depicted as numerical surfaces for the behavior of the optical properties. © 2009.
Start page
1807
End page
1814
Volume
282
Issue
9
Language
English
OCDE Knowledge area
Óptica
Scopus EID
2-s2.0-62349086472
Source
Optics Communications
ISSN of the container
00304018
Sources of information: Directorio de Producción Científica Scopus