cris.boxmetadata.label.title
Ab initio modelling of spin relaxation lengths in disordered graphene nanoribbons
cris.boxmetadata.label.dateissued
01 browse.startsWith.months.january 2019
cris.boxmetadata.label.accesslevel
open access
cris.boxmetadata.label.resourcetype
journal article
cris.boxmetadata.label.authors
cris.boxmetadata.label.publisher
Royal Society of Chemistry
cris.boxmetadata.label.abstract
The spin-dependent transport properties of armchair graphene nanoribbons in the presence of extrinsic spin-orbit coupling induced by a random distribution of nickel adatoms is studied. By combining a recursive Green's function formalism with density functional theory, we explore the influence of ribbon length and metal adatom concentration on the conductance. At a given length, we observed a significant enhancement of the spin-flip channel around resonances and at energies right above the Fermi level. We also estimate the spin-relaxation length, finding values on the order of tens of micrometers at low Ni adatom concentrations. This study is conducted at singular ribbon lengths entirely from fully ab initio methods, providing indirectly evidence that the Dyakonov-Perel spin relaxation mechanism might be the dominant at low concentrations as well as the observation of oscillations in the spin-polarization.
cris.boxmetadata.label.citationstartpage
26027
cris.boxmetadata.label.citationendpage
26032
cris.boxmetadata.label.volume
21
cris.boxmetadata.label.issue
47
cris.boxmetadata.label.language
English
cris.boxmetadata.label.ocdeknowledgeArea
Ingeniería mecánica
Ingeniería de materiales
cris.boxmetadata.label.doi
cris.boxmetadata.label.scopusidentifier
2-s2.0-85075961263
cris.boxmetadata.label.pubmedidentifier
cris.boxmetadata.label.source
Physical Chemistry Chemical Physics
cris.boxmetadata.label.containerissn
14639076
cris.boxmetadata.label.sponsor
This research received the financial support from the Brazilian agencies CAPES and FAPESP. In particular, A. R. R. acknowledges support from FAPESP grant numbers 2017/02317-2 and 2016/01343-7. W. Y. R. acknowledges support from Coorde-nação de Aperfeiçoamento de Pessoal de Nível Superior-Brasil (CAPES) – Finance Code 001. This work uses the computational resources from GRID-UNESP and CENAPAD/SP.
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